低温等离子体-光催化联合技术处理甲苯的试验研究
Toluene Degradation by Non-thermal Plasma & Photocatalyst
DOI: 10.12677/AEP.2013.31B006, PDF, HTML, 下载: 2,878  浏览: 7,559  科研立项经费支持
作者: 马琳*, 梁文俊, 李坚:北京工业大学环境与能源工程学院, 北京, 中国 100124
关键词: 低温等离子体光催化BaTiO3TiO2正交试验甲苯降解Non-thermal Plasma; Catalytic; BaTiO3; TiO2; Orthogonal Test; Toluene Degradation
摘要: 以挥发性有机污染物(VOCs)代表物质甲苯为去除对象,采用低温等离子体-光催化联合技术对其降解开展研究。比较了催化剂-等离子体反应器及空管(不加催化剂)反应器对甲苯的降解性能异同;通过正交试验考察分析了放电区长度、催化剂填充长度、频率、电压和处理气量五个因素对催化剂-等离子体反应器的甲苯去除效果的影响,确定了甲苯降解的最优工艺条件。
>Non-thermal plasma coupled with photocatalysis was employed to remove toluene which was a representative pollutant of volatile organic compounds (VOCs). The similarities and differences of catalyst-plasma reactor and empty (without catalyst) reactor on the toluene degradation performance were studied. Furthermore, the effect of discharge zone length, catalyst filling length, frequency, applied voltage and gas flow rate on the toluene degradation of catalyst-plasma reactor was investigated. Based on the experimental results, the optimal conditions of toluene degradation were determined.
文章引用:马琳, 梁文俊, 李坚. 低温等离子体-光催化联合技术处理甲苯的试验研究[J]. 环境保护前沿, 2013, 3(1): 20-23. http://dx.doi.org/10.12677/AEP.2013.31B006

参考文献

[1] 秦张峰, 关春梅, 王浩静,等. 有害废气的低温等离子体催化净化应用研究[J]. 燃料化学学报.1999, 12(27): 179-185.
[2] 黄碧纯, 杨岳, 张晓明,等.低温等离子体结合光催化剂TiO2去除甲苯[J]. 华南理工大学学报, 2008, 36(11): 27-32.
[3] 李晶欣, 李坚, 梁文俊,等.低温等离子体联合光催化技术降解甲苯的实验研究[J]. 环境污染与防治, 2011, 33(3): 69-73.
[4] 宁晓宇, 陈红, 耿静,等. 低温等离子体-催化协同空气净化技术研究进展[J]. 科技导报, 2009, 27(6): 97-101.
[5] T. Zhu, J. Li , Y. Q. Jin , et al. Decomposition of benzene by non-thermal plasma processing: photocatalyst and ozone effect. Inter.J. Environmental. Science.Technology. 2008,5(3): 375-384.
[6] 赵雷, 周中平. 低温等离子体技术净化空气中的甲苯[J]. 环境科学研究, 2006, 19(4): 70-73.
[7] 邱作志, 叶代启. 放电等离子体驱动光催化降解甲苯研究[J] .工业催化, 2008, 16(6): 69-74.
[8] A. Rousseau, O. Guaitella, L. Gatilova, et al. Photocatalyst activation in a pulsed low pressure discharge. Applied Physics Letters, 2005, 87(22): 221-501.
[9] Maryamossadat Bozorgtabar, Mehdi Salehi, Rahimipour, et al. Photo-catalytic activity and Photo-absorption of Plasma-sprayed Nano-structured TiO2 Coatings. International Journal of Modern Physics, 2010, 24(31): 6115–6127.
[10] T. Oda. Non-thermal plasma processing for environmental protection: Decomposition of dilute VOCs in air. Journal of Electrostatics, 2003, 57(3-4): 293-311.