水中药物及个人护理品去除技术研究进展
Advances in Removal of Aqueous Pharmaceuticals and Personal Care Products
DOI: 10.12677/AEP.2016.66023, PDF, HTML, XML,  被引量 下载: 2,220  浏览: 5,389  科研立项经费支持
作者: 吴东海*, 陆光华, 林秋红, 刘付立:河海大学浅水湖泊综合治理与资源开发教育部重点实验室,江苏 南京;河海大学环境学院,江苏 南京;王 威, 张 佩:河南省水文水资源局,河南 郑州
关键词: 药物及个人护理品水污染去除技术PPCPs Water Pollution Removal Technology
摘要: 新兴污染物药物及个人护理品(Pharmaceuticals and personal care products, PPCPs)威胁水生生态环境和人类健康,对水中PPCPs的污染控制是当前环境领域内的研究热点。本文通过对现有研究分析,阐述了当前国内外水环境中PPCPs的污染现状,归纳了水中PPCPs的主要去除技术,并展望了该领域进一步的研究方向。
Abstract: Pharmaceuticals and personal care products (PPCPs) are a type of emerging contaminants which affect the aquatic ecosystems and human health. The removal of aqueous PPCPs has been widely investigated in recent years. This paper summarizes the current PPCPs pollution in aquatic envi-ronment and reviews the main treatment technologies. Also, further research emphasis of aqueous PPCPs removal was prospected.
文章引用:吴东海, 陆光华, 林秋红, 刘付立, 王威, 张佩. 水中药物及个人护理品去除技术研究进展[J]. 环境保护前沿, 2016, 6(6): 183-188. http://dx.doi.org/10.12677/AEP.2016.66023

参考文献

[1] 潘潇, 强志民, 王为东. 巢湖东半湖饮用水源区沉积物药品和个人护理品(PPCPs)分布与生态风险[J]. 环境化学, 2016, 35(11): 2234-2244.
[2] 胡洪营, 王超, 郭美婷. 药品和个人护理用品(PPCPs)对环境的污染现状与研究进展[J]. 生态环境, 2005, 14(6): 947-952.
[3] 谢正鑫, 陆光华, 孙丽莎, 袁陆妗, 丁剑楠. 水环境中药物及个人护理品(PPCPs)的生物降解研究进展[J]. 水资源保护, 2013, 29(4): 5-11.
[4] 周宁娟. 典型PPCPs在给水处理系统中的变化规律及调控技术研究[D]: [硕士学位论文]. 上海: 东华大学, 2010.
[5] 张盼伟, 周怀东, 赵高峰, 李昆, 刘巧娜, 任敏, 赵丹丹, 李东佼. 太湖表层沉积物中PPCPs的时空分布特征及潜在风险[J]. 环境科学, 2016, 37(9): 3348-3355.
[6] Ellis, J.B. (2006) Pharmaceutical and Personal Care Products (PPCPs) in Urban Receiving Waters. Environmental Pollution, 144, 184-189. https://doi.org/10.1016/j.envpol.2005.12.018
[7] 林秋红. 电化学/臭氧耦合降解水中PPCPs类有机物研究[D]: [硕士学位论文]. 南京: 河海大学. 2015.
[8] Kosma, C.I., Lambropoulou, D.A. and Albanis, T.A. (2014) Investigation of PPCPs in Wastewater Treatment Plants in Greece: Occurrence, Removal and Environmental Risk Assessment. Science of the Total Environment, 466-467, 421-438. https://doi.org/10.1016/j.scitotenv.2013.07.044
[9] Carmona, E., Andreu, V. and Pico, Y. (2014) Occurrence of Acidic Pharmaceuticals and Personal Care Products in Tuna River Basin: From Waste to Drinking Water. Science of the Total Environment, 484, 53-63. https://doi.org/10.1016/j.scitotenv.2014.02.085
[10] Subedi, B., Codru, N., Dziewulski, D.M., Wilson, L.R., Xue, J.C., Yun, S.H., Braun-Howland, E., Minihane, C. and Kannan, K. (2015) A Pilot Study on the Assessment of Trace Organic Contaminants Including Pharmaceuticals and Personal Care Products from On-Site Wastewater Treatment Systems along Skaneateles Lake in New York State, USA. Water Research, 72, 28-39. https://doi.org/10.1016/j.watres.2014.10.049
[11] Gao, J., O’Brien, J., Du, P., Li, X., Ort, C., Mueller, J.F. and Thai, P.K. (2016) Measuring Selected PPCPs in Wastewater to Estimate the Population in Different Cities in China. Science of the Total Environment, 568, 164-170. https://doi.org/10.1016/j.scitotenv.2016.05.216
[12] 王丹, 隋倩, 赵文涛, 吕树光, 邱兆富, 余刚. 中国地表水环境中药物和个人护理品的研究进展[J]. 科学通报, 2014, 59(9): 743-751.
[13] Cai, M.Q., Wang, R., Feng, L. and Zhang, L.Q. (2015) Determination of Selected Pharmaceuticals in Tap Water and Drinking Water Treatment Plant by High-Performance Liquid Chromatography-Triple Quadrupole Mass Spectrometer in Beijing, China. Environmental Science and Pollution Research, 22, 1854-1867. https://doi.org/10.1007/s11356-014-3473-8
[14] Carballa, M., Omil, F. and Lema, J.M. (2005) Removal of Cosmetic Ingredients and Pharmaceuticals in Sewage Primary Treatment. Water Research, 39, 4790-4796. https://doi.org/10.1016/j.watres.2005.09.018
[15] Suarez, S., Lerna, J.M. and Omil, F. (2009) Pre-Treatment of Hospital Wastewater by Coagulation-Flocculation and Flotation. Bioresource Technology, 100, 2138-2146. https://doi.org/10.1016/j.biortech.2008.11.015
[16] 李淞, 方磊, 张燕. 药物与个人护理用品在给水系统中的存在及去除研究进展[J]. 水处理技术, 2014, 40(4): 1-5.
[17] Wang, J. and Wang, S. (2016) Removal of Pharmaceuticals and Personal Care Products (PPCPs) from Wastewater: A Review. Journal of Environmental Management, 182, 620-640. https://doi.org/10.1016/j.jenvman.2016.07.049
[18] Zhu, Z., Xie, J., Zhang, M., Zhou, Q. and Liu F. (2016) Insight into the Adsorption of PPCPs by Porous Adsorbents: Effect of the Properties of Adsorbents and Adsorbates. Environmental Pollution, 214, 524-531. https://doi.org/10.1016/j.envpol.2016.04.070
[19] 周雪飞, 陈家斌, 张亚雷. 膜处理和活性炭吸附去除水环境中的PPCPs[J]. 给水排水, 2009, 35(s2): 81-84.
[20] 陈家斌, 周雪飞, 张亚雷. 水环境中PPCPs的臭氧氧化和高级氧化技术[J]. 给水排水, 2009, 35(s2): 87-92.
[21] 王涛, 彭道平, 李云祯, 白杨, 贺玉龙, 黄涛. 高铁酸盐(Fe(Ⅵ))氧化去除水中PPCPs的研究进展[J]. 环境工程, 2016, 34(8): 40-44.
[22] Soltermann, F., Abegglen, C., Gotz, C. and von Gunten, U. (2016) Bromide Sources and Loads in Swiss Surface Waters and Their Relevance for Bromate Formation during Wastewater Ozonation. Environmental Science & Technology, 50, 9825-9834. https://doi.org/10.1021/acs.est.6b01142
[23] Huber, M.M., Canonica, S., Park, G.Y. and Von Gunten, U. (2003) Oxidation of Pharmaceuticals during Ozonation and Advanced Oxidation Processes. Environmental Science & Technology, 37, 1016-1024. https://doi.org/10.1021/es025896h
[24] Sui, M.H., Xing, S.C., Sheng, L., Huang, S.H. and Guo, H.G. (2012) Heterogeneous Catalytic Ozonation of Ciprofloxacin in Water with Carbon Nanotube Supported Manganese Oxides as Catalyst. Journal of Hazardous Materials, 227, 227-236. https://doi.org/10.1016/j.jhazmat.2012.05.039
[25] Ikehata, K., Naghashkar, N.J. and Ei-Din, M.G. (2006) Degradation of Aqueous Pharmaceuticals by Ozonation and Advanced Oxidation Processes: A Review. Ozone: Science & Engineering, 28, 353-414. https://doi.org/10.1080/01919510600985937
[26] 秦伟伟, 肖书虎, 宋永会, 曾萍, 程建光, 郭晓春, 王欣. O3/UV协同氧化处理黄连素制药废水[J]. 环境科学研究, 2010, 23(7): 877-881.
[27] Panizza, M. and Cerisola, G. (2009) Direct and Mediated Anodic Oxidation of Organic Pollutants. Chemical Reviews, 109, 6541-6569. https://doi.org/10.1021/cr9001319
[28] Radjenovic, J., Flexer, V., Donose, B.C., Sedlak, D.L. and Keller, J. (2013) Removal of the X-Ray Contrast Media Diatrizoate by Electrochemical Reduction and Oxidation. Environmental Science & Technology, 47, 13686-13694. https://doi.org/10.1021/es403410p
[29] García-Morales, M.A., Roa-Morales, G., Barrera-Díaz, C., Bilyeu, B. and Rodrigo, M.A. (2013) Synergy of Electrochemical Oxidation Using Boron-Doped Diamond (BDD) Electrodes and Ozone (O3) in Industrial Wastewater Treatment. Electrochemistry Communications, 27, 34-37. https://doi.org/10.1016/j.elecom.2012.10.028
[30] Wan, Z. and Wang, J.L. (2016) Ce-Doped Zero-Valent Iron Nanoparticles as a Fenton-Like Catalyst for Degradation of Sulfamethazine. RSC Advances, 6, 103523-103531. https://doi.org/10.1039/C6RA23709F
[31] Liang, R., Luo, S., Jing, F., Shen, L., Qin, N. and Wu, L. (2015) A Simple Strategy for Fabrication of Pd@MIL-100(Fe) Nanocomposite as a Visible-Light-Driven Photocatalyst for the Treatment of Pharmaceuticals and Personal Care Products (PPCPs). Applied Catalysis B: Environmental, 176-177, 240-248. https://doi.org/10.1016/j.apcatb.2015.04.009
[32] Chen, X.J., Vollertsen, J., Nielsen, J.L., Dall, A.G. and Bester K. (2015) Degradation of PPCPs in Activated Sludge from Different WWTPs in Denmark. Ecotoxicology, 24, 2073-2080. https://doi.org/10.1007/s10646-015-1548-z
[33] Carballa, M., Omil, F., Ternes, T. and Lema, J.M. (2007) Fate of Pharmaceutical and Personal Care Products (PPCPs) during Anaerobic Digestion of Sewage Sludge. Water Research, 41, 2139-2150. https://doi.org/10.1016/j.watres.2007.02.012
[34] Zhang, D.Q., Gersberg, R.M., Hua, T., Zhu, J.F., Goyal, M.K., Ng, W.J. and Tan, S.K. (2013) Fate of Pharmaceutical Compounds in Hydroponic Mesocosms Planted with Scirpus validus. Environmental Pollution, 181, 98-106. https://doi.org/10.1016/j.envpol.2013.06.016