关于水处理碳核算实例以及不同N2O排放因子应用研究
Example of Carbon Accounting for Water Treatment and Application Study of Different N2O Emission Factors
DOI: 10.12677/AAC.2022.122009, PDF,  被引量   
作者: 辛 文, 王志远:上海理工大学能源与动力工程学院,上海;杨雪晶:华东理工大学机械与动力工程学院,上海
关键词: 温室气体排放因子污水处理协同控制Greenhouse Gas Emission Factors Wastewater Treatment Synergistic Control
摘要: 对污水处理中的温室气体产生机理进行研究。采用生态环境部推荐的方法,对排放因子进行符合工程实际的调整,以甲醇工业污水处理厂的温室气体排放为例,探究不同N2O排放因子的影响,以及结果差异性。结果表明:污水中污染物去除与温室气体(GHG)有关联机制,COD的削减对应CH4,TN的削减会产生N2O;排放因子对结果影响显著,选择合适排放因子至关重要;从温室气体排放总量上来看,直接排放的总量最大,其次是能耗产生的间接排放。
Abstract: The mechanism of greenhouse gas generation in wastewater treatment was investigated. Using the method recommended by the Ministry of Ecology and Environment, the emission factors were adjusted to meet the engineering reality, and the effect of different N2O emission factors and the variability of the results were investigated with the example of GHG emission from A/O wastewater treatment. The results show that: there is a correlation mechanism between pollutant removal and GHG in wastewater, removal of COD corresponds to CH4, and removal of TN generates N2O; emission factors have a significant impact on the results, and the selection of appropriate emission factors is crucial; in terms of total GHG emissions, direct emissions are the largest, followed by indirect emissions from energy consumption.
文章引用:辛文, 杨雪晶, 王志远. 关于水处理碳核算实例以及不同N2O排放因子应用研究[J]. 分析化学进展, 2022, 12(2): 60-67. https://doi.org/10.12677/AAC.2022.122009

参考文献

[1] Crippa, M., Guizzardi, D., Muntean, M., et al. (2019) EDGAR v5.0 Greenhouse Gas Emissions. European Commission, Joint Research Centre (JRC) [Dataset]. http://data.europa.eu/89h/488dc3de-f072-4810-ab83-47185158ce2a
[2] Climate Watch (2021) GHG Emissions. https://www.climatewatchdata.org/ghg-emissions
[3] Wang, J.H., Zhang, J., Xie, H.J., et al. (2011) Methane Emissions from a Full-Scale A/A/O Wastewater Treatment Plant. Bioresource Technology, 102, 5479-5485.
[Google Scholar] [CrossRef] [PubMed]
[4] 柴宏祥, 杨世琪, 何强, 等. 污水生物处理脱氮工艺的温室气体排放比较[J]. 给水排水, 2014, 40(7): 129-134.
[5] 闫旭, 邱德志, 郭东丽, 等. 中国城镇污水处理厂温室气体排放时空分布特征[J]. 环境科学, 2018, 39(3): 1256-1263.
[6] Yan, X., Qiu, D.Z., Zheng, S.K., et al. (2018) Spatial and Temporal Distribution of Greenhouse Gas Emissions From Municipal Wastewater Treatment Plants in China From 2005 to 2014. Earth’s Future, 7, 340-350.
[Google Scholar] [CrossRef
[7] Zhao, X., Jin, X.K., Guo, W., et al. (2019) China’s Urban Methane Emissions from Municipal Wastewater Treatment Plant. Earth’s Future, 7, 480-490.
[Google Scholar] [CrossRef
[8] 蔡博峰, 高庆先, 李中华, 吴静, 曹东, 刘兰翠. 中国城市污水处理厂甲烷排放因子研究[J]. 中国人口·资源与环境, 2015, 25(4): 118-124.
[9] Shahabadi, M.B., Yerushalmi, L. and Haghighat, F. (2010) Estimation of Greenhouse Gas Generation in Wastewater Treatment Plants—Model Development and Application. Chemosphere, 78, 1085-1092.
[Google Scholar] [CrossRef] [PubMed]
[10] Shahabadi, M.B., Yerushalmi, L. and Haghighat, F. (2009) Impact of Process Design on Greenhouse Gas (GHG) Generation by Wastewater Treatment Plants. Water Research, 43, 2679-2687.
[Google Scholar] [CrossRef] [PubMed]
[11] 杨世琪. 城镇污水处理系统碳核算方法与模型研究[D]: [硕士学位论文]. 重庆: 重庆大学, 2013.
[12] Foley, J., de Haas, D., Yuan, Z.G. and Lant, P. (2010) Nitrous Oxide Generation in Full-Scale Biological Nutrient Removal Wastewater Treatment Plants. Water Research, 44, 831-844.
[Google Scholar] [CrossRef] [PubMed]
[13] 生态环境部办公厅. 城镇污水处理厂污染物去除协同控制温室气体核算技术指南(试行) [EB/OL]. https://www.mee.gov.cn/xxgk2018/xxgk/xxgk06/201804/t20180410_629682.html, 2018-04-08.
[14] IPCC (2019) 2019 Refinement to the 2006 IPCC Guidelines for National Greenhouse Gas Inventories. https://www.ipcc.ch/report/2019-refinement-to-the-2006-ipcc-guidelines-for-national-greenhouse-gas-inventories/
[15] Du, M., Zhu, Q., Wang, X., et al. (2018) Estimates and Predictions of Methane Emissions from Wastewater in China from 2000 to 2020. Earth’s Future, 6, 252-263.
[Google Scholar] [CrossRef
[16] Liao, X.W., Tian, Y.J., Gan, Y.W. and Ji, J.P. (2020) Quantifying Urban Wastewater Treatment Sector’s Greenhouse Gas Emissions Using a Hybrid Life Cycle Analysis Method—An Application on Shenzhen City in China. Science of the Total Environment, 745, Article ID: 141176.
[Google Scholar] [CrossRef] [PubMed]
[17] Peng, S., Piao, S., Bousquet, P., et al. (2016) Inventory of Anthropogenic Methane Emissions in Mainland China from 1980 to 2010. Atmospheric Chemistry and Physics, 16, 14545-14562.
[Google Scholar] [CrossRef
[18] Yang, D., Xu, L., Gao, X., et al. (2018) Inventories and Reduction Scenarios of Urban Waste-Related Greenhouse Gas Emissions for Management Potential. Science of the Total Environment, 626, 727-736.
[Google Scholar] [CrossRef] [PubMed]
[19] 余娇, 赵荣欣,肖连刚, 等. 基于“水-能-碳”关联的城市污水处理系统碳排放研究[J]. 资源科学, 2020, 42(6): 1052-1062.
[20] 张超. SBR工艺处理煤化工废水的研究[D]: [硕士学位论文]. 西安: 西安建筑科技大学, 2014.
[21] 郭恰. IPCC污泥碳排放核算模型中DOC取值的不足与修正[J]. 中国给水排水, 2020, 36(16): 49-53.
[22] Yang, S.S., Yu, X.L., Ding, M.Q., He, L., Cao, G.L., Zhao, L., Tao, Y., Pang, J.W., Bai, S.W. and Ding, J. (2021) Simulating a Combined Lysis-Cryptic and Biological Nitrogen Removal System Treating Domestic Wastewater at Low C/N Ratios Using Artificial Neural Network. Water Research, 189, Article ID: 116576.
[Google Scholar] [CrossRef] [PubMed]
[23] Massoompour, A., Borghei, S. and Raie, M. (2020) Enhancement of Biological Nitrogen Removal Performance Using Novel Carriers Based on the Recycling of Waste Materials. Water Research, 170, Article ID: 115340.
[Google Scholar] [CrossRef] [PubMed]
[24] Tallec, G., Garnier, J. and Gousailles, M. (2006) Nitrogen Removal in a Wastewater Treatment Plant through Biofilters: Nitrous Oxide Emissions during Nitrification and Denitrification. Bioprocess and Biosystems Engineering, 29, 323-333.
[Google Scholar] [CrossRef] [PubMed]
[25] Kampschreur, M.J., Temmink, H., Kleerebezem, R., et al. (2009) Nitrous Oxide Emission during Wastewater Treatment. Water Research, 43, 4093-4103.
[Google Scholar] [CrossRef] [PubMed]
[26] Pijuan, M., Tora, J., Rodriguez-Caballero, A., et al. (2014) Effect of Process Parameters and Operational Mode on Nitrous Oxide Emissions from a Nitritation Reactor Treating Reject Wastewater. Water Research, 49, 23-33.
[Google Scholar] [CrossRef] [PubMed]
[27] 杨凌波, 曾思育, 鞠宇平, 等. 我国城市污水处理厂能耗规律的统计分析与定量识别[J]. 给水排水, 2008, 34(10): 42-45.