Ni43Mn41Co5Sn11合金异质结构薄膜的磁特性及其调制
Magnetic Property and Its Electric-Field Modulation Effect in Ni43Mn41Co5Sn11/PMN-PT Laminate Thin Film
DOI: 10.12677/MS.2023.133018, PDF,    国家自然科学基金支持
作者: 李 赫, 徐宏宇, 林小燕, 叶晴莹, 李智炜, 陈水源*：福建师范大学物理与能源学院，福建省量子调控与新能源材料重点实验室，福建 福州
关键词: Heusler合金；磁电异质结；脉冲激光沉积；磁特性；逆磁电效应； Heusler Alloy； Magnetoelectric Heterojunction； Pulsed Laser Deposition； Magnetic Properties； Converse Magnetoelectric Effect
摘要: 采用脉冲激光沉积法在PMN-PT铁电单晶上沉积Ni43Mn41Co5Sn11合金，制备得到NMCS/Au/PMN-PT复合磁电薄膜。采用X射线衍射仪(XRD)和扫描电镜(SEM)对样品进行结构分析；利用综合物性测量系统(PPMS)和磁电综合测试系统研究了磁特性及电场对磁性的调制作用，实验结果表明，Ni43Mn41Co5Sn11铁磁形状记忆合金在测量温区实现了奥氏体到马氏体的一级相变，伴随着磁性的明显变化；电场对薄膜的磁性有调制作用，即存在逆磁电效应。这一体系中的电场调制磁性具有丰富的基础物理研究意义，在传感、电磁探测和信息存储领域有着潜在应用前景。
Abstract: NMCS/Au/PMN-PT composite magnetoelectric thin film was prepared by pulsed laser deposition. X-ray diffractometer (XRD) and scanning electron microscope (SEM) were used to analyze the structure of the thin film. The magnetic properties of Ni43Mn41Co5Sn11 ferromagnetic shape memory alloy (FSMA) and the modulation effect of electric field on magnetic properties were studied by the Physical Properties Measurement System (PPMS) and the Magnetoelectric Measurement System. The experimental results show that, accompanied by obvious magnetization change, the NMCS alloy processes the first-order phase transition from austenite to martensite in the measured temperature region. The electric field can obviously modulate the magnetism of the film, that is, there exists converse mag-netoelectric effect (CME). The electric-field modulating effect on magnetism in this system has abundant basic physics research significance, and presents potential application prospect in the fields of sensors, electromagnetic detection and information storage.
文章引用：李赫, 徐宏宇, 林小燕, 叶晴莹, 李智炜, 陈水源. Ni43Mn41Co5Sn11合金异质结构薄膜的磁特性及其调制[J]. 材料科学, 2023, 13(3): 143-149. https://doi.org/10.12677/MS.2023.133018

参考文献

[1] Fiebig, M. (2005) Revival of the Magnetoelectric Effect. Journal of Physics D: Applied Physics, 38, R123. [Google Scholar] [CrossRef] 
[2] Eerenstein, W., Mathur, N.D. and Scott, J.F. (2006) Multiferroic and Magnetoelectric Materials. Nature, 442, 759. [Google Scholar] [CrossRef] [PubMed]
[3] Geprägs, S., Brandlmaier, A., Opel, M., et al. (2010) Electric Field Con-trolled Manipulation of the Magnetization in Ni/BaTiO3 Hybrid Structures. Applied Physics Letters, 96, Article ID: 142509. [Google Scholar] [CrossRef] 
[4] Ramesh, R. and Spaldin, N.A. (2007) Multiferroics: Progress and Prospects in Thin Films. Nature Materials, 6, 21-29. [Google Scholar] [CrossRef] [PubMed]
[5] 何泓材, 林元华, 南策文. 多铁性磁电复合薄膜[J]. 科学通报, 2008, 53(10): 1136.
[6] Nan, C.W., Bichurin, M.I., Dong, S., et al. (2008) Multiferroic Magnetoelectric Composites: Histor-ical Perspective, Status, and Future Directions. Journal of Applied Physics, 103, Article ID: 031101. [Google Scholar] [CrossRef] 
[7] You, W.B., Lian, G.J., Yang, L.T., et al. (2023) Direct Imaging of Stress-Induced Magnetic Behavior Transitions. Journal of Materials Science & Technology, 146, 72. [Google Scholar] [CrossRef] 
[8] Lewkowitz, M., Adams, J., Sullivan, N.S., et al. (2023) Direct Observation of Electric Field-Induced Magnetism in a Molecular Magnet. Scientific Reports, 13, Article No. 2769. [Google Scholar] [CrossRef] [PubMed]
[9] 姚一平. 多铁复合材料的磁电耦合及电阻转换效应[D]: [博士学位论文]. 合肥: 中国科学技术大学, 2012.
[10] 郑仁奎, 李晓光. 多铁性磁电复合薄膜研究[J]. 物理学进展, 2013(6): 359-368.
[11] Astrov, D.N. (1960) The Magnetoelectric Effects in Antiferromagnetics. Soviet Physics JETP, 11, 708-709.
[12] Folen, V.J., Rado, G.T. and Stalder, E.W. (1961) Anisotropy of Magnetoelectric Effect in Cr2O3. Physical Review Letters, 6, 607. [Google Scholar] [CrossRef] 
[13] Ascher, E., Rieder, H., Schmid, H., et al. (1966) Some Properties of Ferromagnetoelectric Nickel-Iodine Boracite Ni3B7O13I. Journal of Applied Physics, 18, 1404-1405. [Google Scholar] [CrossRef] 
[14] Cherifi, R.O., Ivanovskaya, V., Phillips, L.C., et al. (2014) Electric-Field Control of Magnetic Order above Room Temperature. Nature Materials, 13, 345-351.
[15] Sahoo, S., Polisetty, S., et al. (2007) Ferroelectric Control of Magnetism in BaTiO3/Fe Heterostructures via Interface Strain Cou-pling. Physical Review B, 76, Article ID: 092108. [Google Scholar] [CrossRef] 
[16] Lahtinen, T.H.E., Tuomi, J.O. and van Dijken, S. (2011) Pattern Transfer and Electric-Field-Induced Magnetic Domain Formation in Multiferroic Heterostructures. Advanced Materials, 23, 3187-3191. [Google Scholar] [CrossRef] [PubMed]
[17] Franke, K.J.A., Van de Wiele, B., Shirahata, Y., et al. (2015) Re-versible Electric-Field-Driven Magnetic Domain-Wall Motion. Physical Review X, 5, Article ID: 011010. [Google Scholar] [CrossRef] 

为你推荐