硅基重构表面上金属初期生长行为研究
Initial Growth Behavior of Metals on Reconstructed Silicon Surfaces
DOI: 10.12677/MS.2019.94053, PDF,   
作者: 张 睿, 胡 蔚, 周颖慧:厦门大学物理系,福建 厦门
关键词: Si(111)成核扫描隧道显微镜Si(111) Ag Sn Nucleation Scanning Tunneling Microscopy
摘要: 本文利用超高真空扫描隧道显微镜,研究了Ag和Sn两种金属在Si(111)衬底的不同重构表面上的初期生长和结构演变过程。通过观察低覆盖度下Ag和Sn在7 × 7表面上的吸附成核,探索有序团簇阵列的制备条件。进一步比较两种金属在各自与硅形成的3×√3重构表面上的生长行为差异,并根据其生长特性提出一种在√3-Sn表面制备单原子层厚Sn覆盖层的方法。
Abstract: In this work, the initial growth and structural evolution of Ag and Sn on reconstructed Si(111) surfaces were investigated under ultrahigh vacuum conditions with scanning tunneling microscopy. We studied the adsorption and nucleation of Ag and Sn on 7 × 7 surface at low coverage, and figured out the preparation condition for ordered Sn cluster arrays. The growth behavior of Ag and Sn on 3×√3 reconstructed surfaces was further compared. In the light of the growth characteristics of Sn on 3×√3-Sn surface, a fabrication method of Sn layer with atomic thickness on Si substrate was proposed.
文章引用:张睿, 胡蔚, 周颖慧. 硅基重构表面上金属初期生长行为研究[J]. 材料科学, 2019, 9(4): 411-417. https://doi.org/10.12677/MS.2019.94053

参考文献

[1] Dabrowski, J. and Mussig, H.J. (2003) Silicon Surfaces and Formation of Interfaces. World Scientific, Singa-pore.
[2] Lai, M.Y. and Wang, Y.L. (2001) Self-Organized Two-Dimensional Lattice of Magic Clusters. Physical Review B, 64, Article ID: 241404. [Google Scholar] [CrossRef
[3] Li, J.L., Jia, J.F., Liang, X.J., Liu, X., Wang, J.Z., Xue, Q.K., Li, Z.Q., Tes, J.S., Zhang, Z.Y. and Zhang, S.B. (2002) Spontaneous Assembly of Perfectly Ordered Identical-Size Nanocluster Arrays. Physical Review Letters, 88, Article ID: 066101. [Google Scholar] [CrossRef
[4] Jia, J.F., Liu, X., Wang, J.Z., Li, J.L., Wang, X.S., Xue, Q.K., Li, Z.Q., Zhang, Z.Y. and Zhang, S.B. (2002) Fabrication and Structural Analysis of Al, Ga, and In Nanocluster Crystals. Physical Review B, 66, Article ID: 165412. [Google Scholar] [CrossRef
[5] Li, S.C., Jia, J.F., Dou, R.F., Xue, Q.K., Batyrev, I.G. and Zhang, S.B. (2004) Borderline Magic Clustering: The Fabrication of Tetravalent Pb Cluster Arrays on Si(111)-7×7 Surfaces. Physical Review Letters, 93, Article ID: 116103. [Google Scholar] [CrossRef
[6] Chang, H.H., Lai, M.Y., Wei, J.H., Wei, C.M. and Wang, Y.L. (2004) Structure Determination of Surface Magic Clusters. Physical Review Letters, 92, Article ID: 066103. [Google Scholar] [CrossRef
[7] Bocîrnea, A.E., Costescu, R.M., Apostol, N.G. and Teo-dorescu, C.M. (2019) Growth of Ag(111) on Si(111) with Nearly Flat Band and Abrupt Interface. Applied Surface Science, 473, 433-441. [Google Scholar] [CrossRef
[8] Qin, H., Gao, Y., Teng, J., Xu, H. and Wu, K. (2010) Laterally Tunable Plasmon Resonance in Confined Biatomic-Layer Ag Nanodisks. Nano Letters, 10, 2961-2964. [Google Scholar] [CrossRef] [PubMed]
[9] Tao, M.L., Tu, Y.B., Sun, K., Ye, J., Hao, S.J., Xiao, H.F., Wang, Y.L., Xie, Z.B. and Wang, J.Z. (2017) STM Study of the Ga Thin Films Grown on Si(111) Surface. Surface Science, 663, 31-34. [Google Scholar] [CrossRef
[10] Teng, J., Zhang, L., Jiang, Y., Guo, J., Guo, Q., Wang, E., Ebert, P., Sakurai, T. and Wu, K. (2010) Catalystlike Behavior of Si Adatoms in the Growth of Monolayer Al Film on Si(111). The Journal of Chemical Physics, 133, Article ID: 014704. [Google Scholar] [CrossRef] [PubMed]
[11] Zhang, C., Chen, G., Wang, K.D., Yang, H.W., Su T., Chan, C.T., Loy, M.M.T. and Xiao, X.D. (2005) Experimental and Theo-retical Investigation of Single Cu, Ag, and Au Atoms Adsorbed on Si(111)-7×7. Physical Review Letters, 94, Article ID: 176104. [Google Scholar] [CrossRef
[12] Xie, Z.X. and Tanaka, K.I. (2001) Tin Atoms Absorbed on a Si(111)-7×7 Surface. Surface Science, 479, 26-32. [Google Scholar] [CrossRef
[13] Yoon, M., Lin, X.F., Chizhov, I., Mai, H. and Willis, R.F. (2001) Self-Assembled Nanodot Arrays on Si(111)-7×7 Surfaces. Physical Review B, 64, Article ID: 085321. [Google Scholar] [CrossRef
[14] Yurtsever, A., Abe, M., Morita, S. and Sugimoto, Y. (2017) Atom Manipulation Method to Substitute Individual Adsorbate Atoms into a Si(111)-(7×7) Substrate at Room Tem-perature. Applied Physics Letters, 111, Article ID: 233102. [Google Scholar] [CrossRef
[15] Zhang, H.M., Gustafsson, J.B. and Johansson, L.S.O. (2006) Surface Atomic Structure of Ag/Si(111)- . Physical Review B, 74, Article ID: 201304. [Google Scholar] [CrossRef
[16] Belianinov, A., Unal, B., Ho, K.-M., Wang, C.-Z., Evans, J.W., Tringides, M.C. and Thiel, P.A. (2011) Nucleation and Growth of Ag Islands on the Phase of Ag on Si(111). Journal of Physics: Condensed Matter, 23, Article ID: 265002. [Google Scholar] [CrossRef] [PubMed]
[17] Profeta, G., Continenza, A., Ottaviano, L., Mannstadt, W. and Freeman, A.J. (2000) Structural and Electronic Properties of the Surface. Physical Review B, 62, 1556. [Google Scholar] [CrossRef
[18] Jäger, M., Brand, C., Weber, A.P., Fanciulli, M., Dil, J.H., Pfnür, H. and Tegenkamp, C. (2018) α-Sn Phase on Si(111): Spin Texture of a Two-Dimensional Mott State. Physical Review B, 98, Article ID: 165422. [Google Scholar] [CrossRef